COR-32-24, COR-3224

2-氨基-5-(4-苯基-1-哌嗪甲基)-2-恶唑啉Chemical Name: 2-Amino-5-(4-phenylpiperazin-1-ylmethyl)-2-oxazoline; 5-(4-Phenylpiperazin-1-ylmethyl)-4,5-dihydrooxazol-2-amine
CAS No. 91595-86-7
项目整合开发状态: Phase II
项目研究机构: Cortial (Originator), Sarget (Licensee)
合成路线:The reaction of phenylpiperazine (I) with epichlorhydrin (II) leads to 1-chloro-3-(1-phenyl-4-piperazinyl)-2-propanol.This intermediate is dehydrohalogenated to 1-(1-phenyl-4-piperazinyl)-2,3-epoxypropane (III) using sodium hydroxide.The epoxide is converted without further purification into the corresponding 4,5-dihydro-5-[(4-phenyl-1-piperazinyl)methyl]-2-oxazolamine (COR3224) by condensation with monosodium cyanamide salt in methanol,which permits the solubilization of all compounds.The amidine group of the oxazoline ring induces a tautomeric amino-imino equilibrium.For COR3224 it has been shown by X-ray crystallography that the amino form is preponderant in the free base,whereas the imino form predominates in salts.
📌 参考资料/链接:
参考文献标题:Novel 2-amino-5-aminomethyl-2-oxazolines
文献作者:Creuzet,M.-H.; Feniou,C.; Jarry,C.; Prat,G.; Pontagnier,H.(Societ?Cortial SA)
参考来源:EP 0106776; FR 2546167

📄 详细内容


合成路线:The reaction of phenylpiperazine (I) with epichlorhydrin (II) leads to 1-chloro-3-(1-phenyl-4-piperazinyl)-2-propanol.This intermediate is dehydrohalogenated to 1-(1-phenyl-4-piperazinyl)-2,3-epoxypropane (III) using sodium hydroxide.The epoxide is converted without further purification into the corresponding 4,5-dihydro-5-[(4-phenyl-1-piperazinyl)methyl]-2-oxazolamine (COR3224) by condensation with monosodium cyanamide salt in methanol,which permits the solubilization of all compounds.The amidine group of the oxazoline ring induces a tautomeric amino-imino equilibrium.For COR3224 it has been shown by X-ray crystallography that the amino form is preponderant in the free base,whereas the imino form predominates in salts.

参考文献标题:COR3224
文献作者:D'Arnoux,C.; Panconi,E.; Descas,P.; Vaugien,B.; Lambrey,B.; Mosser,J.; Jarry,C.; Gomond,P.; Saudubray,F.; Roux,J.
参考来源:Drugs Fut 1991,16(10),893


合成路线:The reaction of phenylpiperazine (I) with epichlorhydrin (II) leads to 1-chloro-3-(1-phenyl-4-piperazinyl)-2-propanol.This intermediate is dehydrohalogenated to 1-(1-phenyl-4-piperazinyl)-2,3-epoxypropane (III) using sodium hydroxide.The epoxide is converted without further purification into the corresponding 4,5-dihydro-5-[(4-phenyl-1-piperazinyl)methyl]-2-oxazolamine (COR3224) by condensation with monosodium cyanamide salt in methanol,which permits the solubilization of all compounds.The amidine group of the oxazoline ring induces a tautomeric amino-imino equilibrium.For COR3224 it has been shown by X-ray crystallography that the amino form is preponderant in the free base,whereas the imino form predominates in salts.

参考文献标题:Crystal and molecular structure of 5-(1-aryl-4-piperazino)-methyl-2-amino-2-oxazolines with antidepressant activity
文献作者:Ouhabi,J.; Jarry,C.; Bosc,J.J.; Carpy,A.
参考来源:Arch Pharm 1990,323157-61


合成路线:The reaction of phenylpiperazine (I) with epichlorhydrin (II) leads to 1-chloro-3-(1-phenyl-4-piperazinyl)-2-propanol.This intermediate is dehydrohalogenated to 1-(1-phenyl-4-piperazinyl)-2,3-epoxypropane (III) using sodium hydroxide.The epoxide is converted without further purification into the corresponding 4,5-dihydro-5-[(4-phenyl-1-piperazinyl)methyl]-2-oxazolamine (COR3224) by condensation with monosodium cyanamide salt in methanol,which permits the solubilization of all compounds.The amidine group of the oxazoline ring induces a tautomeric amino-imino equilibrium.For COR3224 it has been shown by X-ray crystallography that the amino form is preponderant in the free base,whereas the imino form predominates in salts.
参考文献标题:Synthesis and antidepressant activity of 5-(1-aryl-4-piperazino)methyl-2-amino-2-oxazolines
文献作者:Bosc,J.J.; Descas,P.; Carpy,A.; Panconi,E.; Jarry,C.
参考来源:Eur J Med Chem 1992,27(5),437


产品链接: CAS No. 91595-86-7››