Murabutide

莫拉布胺Chemical Name: 2-Acetamido-3-O-[(R)-1-[[(S)-3-carbamoyl-1-carboxypropyl]carbamoyl]ethyl]carbamoyl]ethyl]-2-deoxy-D-glucopyranose butyl ester; N-Acetylmuramyl-L-alanyl-D-glutamine n-butyl ester
CAS No. 74817-61-1
项目整合开发状态: Phase II
项目研究机构: Choay (Originator), Institut Pasteur (Originator)
合成路线:The reaction of N-benzltoxycarbonyl-L-alanine succinimidyl ester (I) with o-glutamine (II) by means of triethylamine in THF water gives benzyloxycarbonyl-L-alanyl-o-glutamine (III),which is esterified with bromobutane and Cs2CO3 in DMF yielding the corresponding butyl ester (IV).Deprotection of (IV) by hydrogenation with H2 over Pd/C in acetic acid affords L-alanyl-D-glutamine n-butyl ester (V),which is condensed with 1-O-benzyl-4,6-O-benzylidene-N-acetylmuramic acid (VI) bv the mixed anhydride method affording 1-O-benzyl-4,6-O-benzylidene-N-acetylmuramyl-L-alanyl-o-glutamine n-butyl ester (VII).Finally,this compound is deprotected by hydrogenation with H2 over Pd/C as before.
📌 参考资料/链接:
参考文献标题:Novel compounds of the muramyl peptide
文献作者:Lefrancier,P.; Parant,M.; Audibert,F.; Chedid,L.; Choay,J.; Lederer,E.(ANVAR (Agence Natl.Valor.Rech.))
参考来源:DD 145274; EP 0006068; ES 481785; FR 2428051; JP 55000392; US 4693998

📄 详细内容


合成路线:The reaction of N-benzltoxycarbonyl-L-alanine succinimidyl ester (I) with o-glutamine (II) by means of triethylamine in THF water gives benzyloxycarbonyl-L-alanyl-o-glutamine (III),which is esterified with bromobutane and Cs2CO3 in DMF yielding the corresponding butyl ester (IV).Deprotection of (IV) by hydrogenation with H2 over Pd/C in acetic acid affords L-alanyl-D-glutamine n-butyl ester (V),which is condensed with 1-O-benzyl-4,6-O-benzylidene-N-acetylmuramic acid (VI) bv the mixed anhydride method affording 1-O-benzyl-4,6-O-benzylidene-N-acetylmuramyl-L-alanyl-o-glutamine n-butyl ester (VII).Finally,this compound is deprotected by hydrogenation with H2 over Pd/C as before.

参考文献标题:Murabutide
文献作者:Castar,J.; Prous,J.
参考来源:Drugs Fut 1986,11(9),750


合成路线:The reaction of N-benzltoxycarbonyl-L-alanine succinimidyl ester (I) with o-glutamine (II) by means of triethylamine in THF water gives benzyloxycarbonyl-L-alanyl-o-glutamine (III),which is esterified with bromobutane and Cs2CO3 in DMF yielding the corresponding butyl ester (IV).Deprotection of (IV) by hydrogenation with H2 over Pd/C in acetic acid affords L-alanyl-D-glutamine n-butyl ester (V),which is condensed with 1-O-benzyl-4,6-O-benzylidene-N-acetylmuramic acid (VI) bv the mixed anhydride method affording 1-O-benzyl-4,6-O-benzylidene-N-acetylmuramyl-L-alanyl-o-glutamine n-butyl ester (VII).Finally,this compound is deprotected by hydrogenation with H2 over Pd/C as before.

合成路线:The bromination of 2,6-dimethoxybenzoic acid (I) with Br2 in dioxane gives 3-bromo-2,6-dimethoxy benzoic acid (II),which is treated with refluxing SOCl2 yielding the corresponding acyl chloride (III).Finally,this compound is condensed with (-)-(S)-1-ethyl 2-(aminomethyl)pyrrolidine (IV).
参考文献标题:Potential neuroleptic agents.2,6-dialkoxybenzamide derivatives with potent dopamine receptor blocking activities
文献作者:Florvall,L.; Ogren,S.O.
参考来源:J Med Chem 1982,25(11),1280


产品链接: CAS No. 74817-61-1››