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Tolrestatin, Tolrestat, AY-27773, Alrestin, Lorestat, Alredase

托雷斯萘Chemical Name: N-[6-Methoxy-5-(trifluoromethyl)-1-naphthylthiocarbonyl]-N-methylglycine
CAS No. 82964-04-3
项目整合开发状态: Withdrawn
项目研究机构: Wyeth Pharmaceuticals (Originator), Recordati (Licensee)
合成路线:The reaction of 6-methoxy-5-(trifluoromethyl)naphthalene-1-carboxylic acid (I) with SOCl2 in refluxing DMF gives the corresponding acyl chloride (II),which is condensed with methyl N-methylglycinate (III) by means of hydroxybenzotriazole and dicyclohexylcarbodiimide in DMF yielding methyl N-[[5-(trifluoromethyl)-6-methoxy-1-naphthyl]carbonyl]-N-methylglycinate (IV).The reaction of (IV) with P2S5 refluxing pyridine affords methyl N-[[5-(trifluoromethyl)-6-methoxy-1-naphthyl]thioxomethyl]-N-methylglycinate (V),which is finally hydrolyzed with NaOH in methanol water.The synthesis of [14C]-labeled tolrestat has also been described.
📌 参考资料/链接:
参考文献标题:N-Naphtoylglycine derivatives
文献作者:Sestanj,K.; Abraham,N.A.; Bellini,F.; Treasurywala,A.; Humber,L.G.(Ayerst Laboratories Inc.)
参考来源:EP 0059596; JP 570158756; US 4391825

📄 详细内容


合成路线:The reaction of 6-methoxy-5-(trifluoromethyl)naphthalene-1-carboxylic acid (I) with SOCl2 in refluxing DMF gives the corresponding acyl chloride (II),which is condensed with methyl N-methylglycinate (III) by means of hydroxybenzotriazole and dicyclohexylcarbodiimide in DMF yielding methyl N-[[5-(trifluoromethyl)-6-methoxy-1-naphthyl]carbonyl]-N-methylglycinate (IV).The reaction of (IV) with P2S5 refluxing pyridine affords methyl N-[[5-(trifluoromethyl)-6-methoxy-1-naphthyl]thioxomethyl]-N-methylglycinate (V),which is finally hydrolyzed with NaOH in methanol water.The synthesis of [14C]-labeled tolrestat has also been described.

参考文献标题:Tolrestat
文献作者:Castar,J.; Serradell,M.N.
参考来源:Drugs Fut 1984,9(9),670


合成路线:The reaction of 6-methoxy-5-(trifluoromethyl)naphthalene-1-carboxylic acid (I) with SOCl2 in refluxing DMF gives the corresponding acyl chloride (II),which is condensed with methyl N-methylglycinate (III) by means of hydroxybenzotriazole and dicyclohexylcarbodiimide in DMF yielding methyl N-[[5-(trifluoromethyl)-6-methoxy-1-naphthyl]carbonyl]-N-methylglycinate (IV).The reaction of (IV) with P2S5 refluxing pyridine affords methyl N-[[5-(trifluoromethyl)-6-methoxy-1-naphthyl]thioxomethyl]-N-methylglycinate (V),which is finally hydrolyzed with NaOH in methanol water.The synthesis of [14C]-labeled tolrestat has also been described.

参考文献标题:N-[[5-(Trifluoromethyl)-6-methoxy-1-naphthalenyl]thioxomethyl]-N-methylglycine (tolrestat),a potent,orally active aldose reductase inhibitor
文献作者:Sestanj,K.; Bellini,F.; Fung,S.; Abraham,N.A.; Treasurywala,A.; Humber,L.G.; Simar-Duquesne,N.; Dvornik,D.
参考来源:J Med Chem 1984,27(43),255-256


合成路线:The reaction of 6-methoxy-5-(trifluoromethyl)naphthalene-1-carboxylic acid (I) with SOCl2 in refluxing DMF gives the corresponding acyl chloride (II),which is condensed with methyl N-methylglycinate (III) by means of hydroxybenzotriazole and dicyclohexylcarbodiimide in DMF yielding methyl N-[[5-(trifluoromethyl)-6-methoxy-1-naphthyl]carbonyl]-N-methylglycinate (IV).The reaction of (IV) with P2S5 refluxing pyridine affords methyl N-[[5-(trifluoromethyl)-6-methoxy-1-naphthyl]thioxomethyl]-N-methylglycinate (V),which is finally hydrolyzed with NaOH in methanol water.The synthesis of [14C]-labeled tolrestat has also been described.
参考文献标题:Synthesis of [14C]-labelled tolrestat (N-[[5-(trifluoromethyl)-6-methoxy-1-naphthalenyl]-[14C]thioxomethyl]-N-methylglycine
文献作者:Hicks,D.R.
参考来源:J Label Compd Radiopharm 1984,21(3),229-236


产品链接: CAS No. 82964-04-3››