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Ganirelix acetate, Org-37462, RS-26306, Antagon, Orgalutran

加尼瑞克 Chemical Name: N-Acetyl-3-(2-naphthyl)-D-alanyl-4-chloro-D-phenylalanyl-3-(3-pyridinyl)-D-alanyl-L-seryl-L-tyrosyl-N6-[(ethylamino)(ethylimino)methyl]-D-lysyl-L-leucyl-N6-[(ethylamino)(ethylimino)methyl]-L-lysyl-L-prolyl-D-alaninamide diacetate; N-Acetyl-3-(2-naphthyl)-D-alanyl-4-chloro-D-phenylalanyl-3-(3-pyridyl)-D-alanyl-L-seryl-L-tyrosyl-Nomega,N'omega-diethyl-D-homoarginyl-L-leucyl-Nomega,N'omega-diethyl-L-homoarginyl-L-prolyl-D-alaninamide diacetate
CAS No. 129311-55-3, 124904-93-4 (free base)
项目整合开发状态: Launched-2000
项目研究机构: Roche (Originator), Organon (Licensee)
合成路线:The synthesis of ganirelix was performed using usual solid-state peptide synthesis with a Beckman 990 or a 5.0 L Vega 296 automated solid-phase peptide synthesizer.The synthesis was initiated by condensation of chloromethylated polystyrene/divinylbenzene resin (Merrifieled resin) (II) with Boc-D-alanine (I) by means of cesium carbonate,giving Boc-D-ala-RESIN (III),which was submitted to successive cycles of deprotection with TFA or HCl and addition of a new protected amino acid by means of DCC or HOBt.The following amino acids were added successively: Boc-L-proline (IV),Nalpha-Boc-Nomega,N'omega-diethyl-L-homoarginine (VI),Boc-L-leucine (VIII),Nalpha-Boc-Nomega,N'omega-diethyl-D-homoarginine (X) and Boc-L-tyrosine (XII),yielding successively the peptide resins (V),(VII),(IX),(XI) and (XIII).

合成路线:The synthesis of ganirelix was performed using usual solid-state peptide synthesis with a The following amino acids were added successively to intermediate (XIII): N-Boc-O-benzyl-L-serine (XIV),Boc-(3-pyridyl)-D-alanine (XVI) and Boc-4-chloro-D-phenylalanine (XVIII),yielding successively the peptide resins (XV),(XVII) and (XIX).

合成路线:The amino acid Boc-(2-naphthyl)-D-alanine (XX) were added to intermediate (XIX),yielding the peptide resin (XXI).When the integration of amino acids was completed,the peptide resin (XXI) was deprotected with TFA,acetylated with acetic anhydride and finally treated with ammonia in methanol in order to eliminate the resin matrix and form the final amide group.
📌 参考资料/链接:
参考文献标题:Nonapeptide and decapeptide analogs of LHRH as LHRH antagonists
文献作者:Nestor,J.J.Jr.; Vickery,B.H.(Syntex (USA),Inc.)
参考来源:EP 0277829; JP 1988201199; US 4801577

📄 详细内容


合成路线:The synthesis of ganirelix was performed using usual solid-state peptide synthesis with a Beckman 990 or a 5.0 L Vega 296 automated solid-phase peptide synthesizer.The synthesis was initiated by condensation of chloromethylated polystyrene/divinylbenzene resin (Merrifieled resin) (II) with Boc-D-alanine (I) by means of cesium carbonate,giving Boc-D-ala-RESIN (III),which was submitted to successive cycles of deprotection with TFA or HCl and addition of a new protected amino acid by means of DCC or HOBt.The following amino acids were added successively: Boc-L-proline (IV),Nalpha-Boc-Nomega,N'omega-diethyl-L-homoarginine (VI),Boc-L-leucine (VIII),Nalpha-Boc-Nomega,N'omega-diethyl-D-homoarginine (X) and Boc-L-tyrosine (XII),yielding successively the peptide resins (V),(VII),(IX),(XI) and (XIII).

合成路线:The synthesis of ganirelix was performed using usual solid-state peptide synthesis with a The following amino acids were added successively to intermediate (XIII): N-Boc-O-benzyl-L-serine (XIV),Boc-(3-pyridyl)-D-alanine (XVI) and Boc-4-chloro-D-phenylalanine (XVIII),yielding successively the peptide resins (XV),(XVII) and (XIX).

合成路线:The amino acid Boc-(2-naphthyl)-D-alanine (XX) were added to intermediate (XIX),yielding the peptide resin (XXI).When the integration of amino acids was completed,the peptide resin (XXI) was deprotected with TFA,acetylated with acetic anhydride and finally treated with ammonia in methanol in order to eliminate the resin matrix and form the final amide group.

参考文献标题:LHRH antagonist analogs and 19-nor-progestational steroids for therapy
文献作者:Vickery,B.H.(Syntex (USA),Inc.)
参考来源:EP 0301850


合成路线:The synthesis of ganirelix was performed using usual solid-state peptide synthesis with a Beckman 990 or a 5.0 L Vega 296 automated solid-phase peptide synthesizer.The synthesis was initiated by condensation of chloromethylated polystyrene/divinylbenzene resin (Merrifieled resin) (II) with Boc-D-alanine (I) by means of cesium carbonate,giving Boc-D-ala-RESIN (III),which was submitted to successive cycles of deprotection with TFA or HCl and addition of a new protected amino acid by means of DCC or HOBt.The following amino acids were added successively: Boc-L-proline (IV),Nalpha-Boc-Nomega,N'omega-diethyl-L-homoarginine (VI),Boc-L-leucine (VIII),Nalpha-Boc-Nomega,N'omega-diethyl-D-homoarginine (X) and Boc-L-tyrosine (XII),yielding successively the peptide resins (V),(VII),(IX),(XI) and (XIII).

合成路线:The synthesis of ganirelix was performed using usual solid-state peptide synthesis with a The following amino acids were added successively to intermediate (XIII): N-Boc-O-benzyl-L-serine (XIV),Boc-(3-pyridyl)-D-alanine (XVI) and Boc-4-chloro-D-phenylalanine (XVIII),yielding successively the peptide resins (XV),(XVII) and (XIX).

合成路线:The amino acid Boc-(2-naphthyl)-D-alanine (XX) were added to intermediate (XIX),yielding the peptide resin (XXI).When the integration of amino acids was completed,the peptide resin (XXI) was deprotected with TFA,acetylated with acetic anhydride and finally treated with ammonia in methanol in order to eliminate the resin matrix and form the final amide group.

参考文献标题:Temporary minimal protection synthesis of LH-RH analogs
文献作者:Nestor,J.J.Jr.; McClure,N.L.(Syntex (USA),Inc.)
参考来源:EP 0443532; JP 1992211096; US 5212288


合成路线:The synthesis of ganirelix was performed using usual solid-state peptide synthesis with a Beckman 990 or a 5.0 L Vega 296 automated solid-phase peptide synthesizer.The synthesis was initiated by condensation of chloromethylated polystyrene/divinylbenzene resin (Merrifieled resin) (II) with Boc-D-alanine (I) by means of cesium carbonate,giving Boc-D-ala-RESIN (III),which was submitted to successive cycles of deprotection with TFA or HCl and addition of a new protected amino acid by means of DCC or HOBt.The following amino acids were added successively: Boc-L-proline (IV),Nalpha-Boc-Nomega,N'omega-diethyl-L-homoarginine (VI),Boc-L-leucine (VIII),Nalpha-Boc-Nomega,N'omega-diethyl-D-homoarginine (X) and Boc-L-tyrosine (XII),yielding successively the peptide resins (V),(VII),(IX),(XI) and (XIII).

合成路线:The synthesis of ganirelix was performed using usual solid-state peptide synthesis with a The following amino acids were added successively to intermediate (XIII): N-Boc-O-benzyl-L-serine (XIV),Boc-(3-pyridyl)-D-alanine (XVI) and Boc-4-chloro-D-phenylalanine (XVIII),yielding successively the peptide resins (XV),(XVII) and (XIX).

合成路线:The amino acid Boc-(2-naphthyl)-D-alanine (XX) were added to intermediate (XIX),yielding the peptide resin (XXI).When the integration of amino acids was completed,the peptide resin (XXI) was deprotected with TFA,acetylated with acetic anhydride and finally treated with ammonia in methanol in order to eliminate the resin matrix and form the final amide group.

参考文献标题:Ganirelix Acetate
文献作者:Castar,J.; Leeson,P.; Rabasseda,X.
参考来源:Drugs Fut 1999,24(4),393


合成路线:The synthesis of ganirelix was performed using usual solid-state peptide synthesis with a Beckman 990 or a 5.0 L Vega 296 automated solid-phase peptide synthesizer.The synthesis was initiated by condensation of chloromethylated polystyrene/divinylbenzene resin (Merrifieled resin) (II) with Boc-D-alanine (I) by means of cesium carbonate,giving Boc-D-ala-RESIN (III),which was submitted to successive cycles of deprotection with TFA or HCl and addition of a new protected amino acid by means of DCC or HOBt.The following amino acids were added successively: Boc-L-proline (IV),Nalpha-Boc-Nomega,N'omega-diethyl-L-homoarginine (VI),Boc-L-leucine (VIII),Nalpha-Boc-Nomega,N'omega-diethyl-D-homoarginine (X) and Boc-L-tyrosine (XII),yielding successively the peptide resins (V),(VII),(IX),(XI) and (XIII).

合成路线:The synthesis of ganirelix was performed using usual solid-state peptide synthesis with a The following amino acids were added successively to intermediate (XIII): N-Boc-O-benzyl-L-serine (XIV),Boc-(3-pyridyl)-D-alanine (XVI) and Boc-4-chloro-D-phenylalanine (XVIII),yielding successively the peptide resins (XV),(XVII) and (XIX).

合成路线:The amino acid Boc-(2-naphthyl)-D-alanine (XX) were added to intermediate (XIX),yielding the peptide resin (XXI).When the integration of amino acids was completed,the peptide resin (XXI) was deprotected with TFA,acetylated with acetic anhydride and finally treated with ammonia in methanol in order to eliminate the resin matrix and form the final amide group.
参考文献标题:Temporary serine protection in solid phase synthesis of LH-RH analogs
文献作者:Arzeno,H.B.; Bingenheimer,W.; Blanchette,R.; Morgans,D.J.; Robinson,J.3rd
参考来源:Int J Pept Protein Res 1993,41(4),342


产品链接: CAS No. 129311-55-3››

产品链接: CAS No.124904-93-4››