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Piretanide, Hoe-118, Eurelix, Tauliz, Arelix

吡咯他尼Chemical Name: 4-Phenoxy-3-(1-pyrrolidinyl)-5-sulfamoylbenzoic acid; 3-(Aminosulfonyl)-4-phenoxy-5-(1-pyrrolidinyl)benzoic acid
CAS No. 55837-27-9
项目整合开发状态: Launched-1981
项目研究机构: Aventis Pharma (Originator)
合成路线:The esterification of 4-phenoxy-3-nitro-5-sulfamoylbenzoic acid (I) with methanol and H2SO4 gives the corresponding methyl ester (II),which is reduced with H2 over Raney-Ni in methanol yielding methyl 4-phenoxy-3-amino-5-sulfamoylbenzoate (III).The condensation of (III) with succinic anhydride (B) or succinoyl chloride (A) by means of pyridine in refluxing dioxane affords methyl 4-phenoxy-3N-succinimido-5-sulfamoylbenzoate (IV),which is reduced with borontrifluoride ethearate and NaBH4 in diglyme giving methyl 4-phenoxy-3-(1-pyrrolidinyl)-5-sulfamoylbenzoate (V).Finally,this compound is hydrolyzed with NaOH in water.
📌 参考资料/链接:
参考文献标题:Piretanide
文献作者:Hillier,K.; Castar,J.
参考来源:Drugs Fut 1977,2(6),393

📄 详细内容


合成路线:The esterification of 4-phenoxy-3-nitro-5-sulfamoylbenzoic acid (I) with methanol and H2SO4 gives the corresponding methyl ester (II),which is reduced with H2 over Raney-Ni in methanol yielding methyl 4-phenoxy-3-amino-5-sulfamoylbenzoate (III).The condensation of (III) with succinic anhydride (B) or succinoyl chloride (A) by means of pyridine in refluxing dioxane affords methyl 4-phenoxy-3N-succinimido-5-sulfamoylbenzoate (IV),which is reduced with borontrifluoride ethearate and NaBH4 in diglyme giving methyl 4-phenoxy-3-(1-pyrrolidinyl)-5-sulfamoylbenzoate (V).Finally,this compound is hydrolyzed with NaOH in water.

参考文献标题:5-Sulfamoylbenzoic acid derivatives carrying a heterocyclic substituent
文献作者:Bormann,D.; et al.
参考来源:DE 2419970; FR 2324298; GB 1504505; US 4010273


合成路线:The esterification of 4-phenoxy-3-nitro-5-sulfamoylbenzoic acid (I) with methanol and H2SO4 gives the corresponding methyl ester (II),which is reduced with H2 over Raney-Ni in methanol yielding methyl 4-phenoxy-3-amino-5-sulfamoylbenzoate (III).The condensation of (III) with succinic anhydride (B) or succinoyl chloride (A) by means of pyridine in refluxing dioxane affords methyl 4-phenoxy-3N-succinimido-5-sulfamoylbenzoate (IV),which is reduced with borontrifluoride ethearate and NaBH4 in diglyme giving methyl 4-phenoxy-3-(1-pyrrolidinyl)-5-sulfamoylbenzoate (V).Finally,this compound is hydrolyzed with NaOH in water.
参考文献标题:Piretanide (Hoe 118) a new high ceiling salidiuretic
文献作者:Merkel,W.; et al.
参考来源:Eur J Med Chem 1976,11(5),399


产品链接: CAS No. 55837-27-9››